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AbstractDue to the lack of any magnetic order down to 1.7 K in the parent bulk compound NdNiO2, the recently discovered 9–15 K superconductivity in the infinite‐layer Nd0.8Sr0.2NiO2 thin films has provided an exciting playground for unearthing new superconductivity mechanisms. Herein, the successful synthesis of a series of superconducting Nd0.8Sr0.2NiO2 thin films ranging from 8 to 40 nm is reported. The large exchange bias effect is observed between the superconducting Nd0.8Sr0.2NiO2 films and a thin ferromagnetic layer, which suggests the existence of the antiferromagnetic order. Furthermore, the existence of the antiferromagnetic order is evidenced by X‐ray magnetic linear dichroism measurements. These experimental results are fundamentally critical for the current field.