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Royal Society of Chemistry, Journal of Materials Chemistry C Materials for optical and electronic devices, 30(7), p. 9184-9194, 2019

DOI: 10.1039/c9tc02742d

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Revealing resonance effects and intramolecular dipole interactions in the positional isomers of benzonitrile-core thermally activated delayed fluorescence materials

Journal article published in 2019 by Nadzeya A. Kukhta ORCID, Heather F. Higginbotham, Tomas Matulaitis ORCID, Andrew Danos ORCID, Aisha N. Bismillah ORCID, Nils Haase, Marc K. Etherington ORCID, Dmitry S. Yufit ORCID, Paul R. McGonigal ORCID, Juozas Vidas Gražulevičius ORCID, Andrew P. Monkman ORCID
This paper was not found in any repository, but could be made available legally by the author.
This paper was not found in any repository, but could be made available legally by the author.

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Abstract

Rather than donor–acceptor dihedral angles, the TADF performance of DMAC–BZN positional isomers is instead controlled by differences in acceptor strength arising from π-system electron density – along with a through-space dipole interaction.